Research On the Application and The Interface Problem of Solid-State Batteries

Authors

  • Hanshen Chen HD Shanghai School, Shanghai, China

DOI:

https://doi.org/10.54097/kkdyst24

Keywords:

lithium-ion batteries, solid state electrolytes, interface problem.

Abstract

Solid-state electrolytes (SSEs), the substitutes of liquid electrolytes which can create greater safety by preventing the penetration from lithium dendrites. However, there are still some defects, as the solid-solid contact may cause interface problems where gaps are formed between electrodes and SSEs. The interface issue can harshly affect the performance of batteries such as overpotential, electrical conductivity, and cycle life. By tackling such issues, traditional lithium-ion batteries can be completely replaced by solid-state batteries due to the outstanding performance of efficiency and capacity. So the solutions are listed by classifying SSEs into different types This essay provides new perspectives and ideas for the researchers by reviewing research on solid-state batteries.

Downloads

Download data is not yet available.

References

[1] M.Stanley Whittingham, Lithium Batteries and Cathode Materials. Chemical Reviews, 2004, 104(10): 4271-4302.

[2] Yang Zhao, Kelly Zheng, Xueliang Sun, Addressing Interfacial Issues in Liquid-Based and Solid-State Batteries by Atomic and Molecular Layer Deposition. Joule, 2018, 2(12): 2583-2604.

[3] William D. Richards, Lincoln J. Miara, Yan Wang, et al. Interface Stability in Solid-State Batteries. Chemistry of Materials, 2016, 28(1): 266-273.

[4] Weizhuo Li, Zhiming Bao, Qing Du, et al. Open-Source CFD Elucidating Mechanism of 3D Pillar Electrode in Improving All-Solid-State Battery Performance. Advanced Science, 2022, 9(13): 2105454.

[5] Feipeng Zhao, Qian Sun, Chuang Yu, et al. Ultra-stable Anode Interface Achieved by Fluorinating Electrolytes for All-Solid-State Li Metal Batteries. ACS Energy Letters, 2020, 5(4):1035–1043.

[6] Shuai Chen, Chuang Yu, et al. Research Progress of Lithium Metal Halide Solid Electrolytes. Acta Physico-Chimica Sinica, 2023, 39(8): 2210032.

[7] Zhigang Xue, Dan He, et al. PEO-based electrolytes blended with star polymers with precisely imprinted polymeric pseudo-crown ether cavities for alkali metal ion batteries. Journal of Membrane Science, 2019, 576(15): 182-189.

[8] Yuhang Zhang, Wei Lu, Lina Cong, et al. Cross-linking network based on Poly(ethylene oxide): Solid polymer electrolyte for room temperature lithium battery. Journal of Power Sources, 2019, 420(30): 63-72.

[9] Yi Cao, Pengjian Zuo, Shuaifeng Lou, et al. A quasi-solid-state Li–S battery with high energy density, superior stability and safety. Journal of Materials Chemistry A, 2019, 7(11): 6533-6542.

[10] Yutao Li, Xi Chen, Andrei Dolocan, et al. Garnet Electrolyte with an Ultralow Interfacial Resistance for Li-Metal Batteries. Journal of the American Chemical Society, 2018, 140(20): 6448–6455.

[11] Hanyu Huo, Yue Chen, Ning Zhao, et al. In-situ formed Li2CO3-free garnet/Li interface by rapid acid treatment for dendrite-free solid-state batteries. Nano Energy, 2019, 61, 119-125.

[12] Hanyu Huo, Jing Luo, Venkataraman Thangadurai, et al. Li2CO3: A Critical Issue for Developing Solid Garnet Batteries. ACS Energy Letters, 2019, 5(1): 252-262.

[13] Lingjun Huang, Ling Zhang, Jiaying Bi, et al. An Insight into Halide Solid-State Electrolytes: Progress and Modification Strategies, Energy Material Advances, 2024, 4, 0092.

[14] Fuqian Liu, Lu Gao, Zhipeng Zhang, et al. Interfacial Challenges, processing strategies, and composite applications for high voltage all-solid-state lithium batteries based on halide and sulfide solid-state electrolytes. Energy Storage Materials, 2024, 64, 103072.

Downloads

Published

28-10-2025

How to Cite

Chen, H. (2025). Research On the Application and The Interface Problem of Solid-State Batteries. Highlights in Science, Engineering and Technology, 157, 33-38. https://doi.org/10.54097/kkdyst24